Effect of nanostructuring of coprecipitated precursors on the morphology and scintillation properties of multication ceramics with a garnet structure
Nanosistemy: fizika, himiâ, matematika, Tome 15 (2024) no. 6, pp. 893-901
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Single-phase polycrystalline samples of the (Gd,Y)$_3$Al$_2$Ga$_3$O$_{12}$:Ce,Tb composition with a garnet structural type were obtained. Using various approaches to the preparation of the initial powders of hydroxycarbonate precursors and compaction methods, the grain size of the ceramics was varied. The scanning electron microscopy method was used to establish the features of the microstructure of the initial powders with different processing temperatures and the microstructure of the resulting ceramics. It is shown that an increase in the grain size of the ceramics and a decrease in the residual porosity gives a noticeable increase in optical transparency in the visible region of the spectrum, in which Ce$^{3+}$ and Tb$^{3+}$ ions emit during scintillation. The effect of intergrain boundaries of the ceramics on the diffusion features of nonequilibrium carriers, electrons and holes, as well as excitons formed during the absorption of ionizing radiation on the scintillation yield and energy resolution is considered.
Keywords:
precursor, ceramics, garnet, light yield.
Mots-clés : microstructure, scintillation
Mots-clés : microstructure, scintillation
@article{NANO_2024_15_6_a15,
author = {Valentina G. Smyslova and Vasiliy M. Retivov and Valery V. Dubov and Lidia V. Ermakova and Vladimir K. Ivanov and Petr V. Karpyuk and Ilya Yu. Komendo and Daria E. Lelekova and Vitaly A. Mechinsky and Andrey N. Vasil'ev and Artemii S. Ilyushin and Petr S. Sokolov and Mikhail V. Korzhik},
title = {Effect of nanostructuring of coprecipitated precursors on the morphology and scintillation properties of multication ceramics with a garnet structure},
journal = {Nanosistemy: fizika, himi\^a, matematika},
pages = {893--901},
year = {2024},
volume = {15},
number = {6},
language = {en},
url = {http://geodesic.mathdoc.fr/item/NANO_2024_15_6_a15/}
}
TY - JOUR AU - Valentina G. Smyslova AU - Vasiliy M. Retivov AU - Valery V. Dubov AU - Lidia V. Ermakova AU - Vladimir K. Ivanov AU - Petr V. Karpyuk AU - Ilya Yu. Komendo AU - Daria E. Lelekova AU - Vitaly A. Mechinsky AU - Andrey N. Vasil'ev AU - Artemii S. Ilyushin AU - Petr S. Sokolov AU - Mikhail V. Korzhik TI - Effect of nanostructuring of coprecipitated precursors on the morphology and scintillation properties of multication ceramics with a garnet structure JO - Nanosistemy: fizika, himiâ, matematika PY - 2024 SP - 893 EP - 901 VL - 15 IS - 6 UR - http://geodesic.mathdoc.fr/item/NANO_2024_15_6_a15/ LA - en ID - NANO_2024_15_6_a15 ER -
%0 Journal Article %A Valentina G. Smyslova %A Vasiliy M. Retivov %A Valery V. Dubov %A Lidia V. Ermakova %A Vladimir K. Ivanov %A Petr V. Karpyuk %A Ilya Yu. Komendo %A Daria E. Lelekova %A Vitaly A. Mechinsky %A Andrey N. Vasil'ev %A Artemii S. Ilyushin %A Petr S. Sokolov %A Mikhail V. Korzhik %T Effect of nanostructuring of coprecipitated precursors on the morphology and scintillation properties of multication ceramics with a garnet structure %J Nanosistemy: fizika, himiâ, matematika %D 2024 %P 893-901 %V 15 %N 6 %U http://geodesic.mathdoc.fr/item/NANO_2024_15_6_a15/ %G en %F NANO_2024_15_6_a15
Valentina G. Smyslova; Vasiliy M. Retivov; Valery V. Dubov; Lidia V. Ermakova; Vladimir K. Ivanov; Petr V. Karpyuk; Ilya Yu. Komendo; Daria E. Lelekova; Vitaly A. Mechinsky; Andrey N. Vasil'ev; Artemii S. Ilyushin; Petr S. Sokolov; Mikhail V. Korzhik. Effect of nanostructuring of coprecipitated precursors on the morphology and scintillation properties of multication ceramics with a garnet structure. Nanosistemy: fizika, himiâ, matematika, Tome 15 (2024) no. 6, pp. 893-901. http://geodesic.mathdoc.fr/item/NANO_2024_15_6_a15/